Development of wrinkled thin film devices for stretchable electronics.

Abstract

Stretchable electronics are soft and light weight. Compared with conventional wafer-based electronics, which are rigid and planar, stretchable electronics can conform to curved surfaces and movable parts. The unique properties of stretchable electronics enable their integration with the human body, and open the door for ever more compelling applications, such as advanced surgical tools, wearable monitoring electronics, implantable prosthesis, and many others. However, the development of stretchable electronics is still at an early stage since their mechanical robustness and electrical performance are still far from satisfying.

In this work, I have developed a method to fabricate thin film stretchable devices by solvent-assisted transfer of wrinkled thin films from rigid polystyrene (PS) substrates to elastomeric polydimethylsiloxane (PDMS) substrates. Using this approach, structured thin films containing multiple materials and hybrid structures could be lifted off simultaneously, facilitating the fabrication of stretchable thin film devices. With this approach, I have built corrosion-resistant stretchable electrodes, stretchable thin film heaters, and stretchable thin film inductors. These applications demonstrate the simplicity and effectiveness of this stretchable electronics fabrication strategy. Finally, I made the first step towards fabricating dye-sensitized solar cells (DSSCs) with room temperature processes, including the preparation of mesoporous TiO2 layers through mechanical compression and the integration of an interdigitated electrode that was fabricated solely by bench-top patterning, alignment, and sputtering deposition. These steps lay the foundation for the future development of stretchable DSSC. I anticipate that the fabricated stretchable thin films electronic components will contribute to the advancement of wearable and implantable electronics.